LMS Volume 33 Issue 3 | Page 18

18  LMS  Issue 3 | 2014 Chromatography & HPLC Break Free from Routine Sample Prep T he Samplicity® filtration system is an innovative new technology that provides a convenient, high throughput alternative to syringe-tip filters when preparing samples for chromatography. This is the f irst vacuum-driven system designed with the f lexibility to filter one to eight samples directly into standard HPLC vials. Just attach a vacuum pump, load samples with a standard pipette and flip the lever to recover particulate-free samples - even those with high viscosity or particulates - in seconds. In addition, the system has a low hold-up volume, which allows processing of samples as small as 300µl. The overall trend in chromatography is to do more with less. More samples, more complex analyses, more analysis per sample with less volume, lower concentrations, in less time, with fast analytical techniques such as ultrahigh pressure liquid chromatography (UHPLC). Even though efficient, high quality sample preparation is crucial in obtaining reliable data from these ultrasensitive techniques, there have been few recent advances in sample preparation technology. As a result, it is often sample preparation, not analysis that is the rate-limiting bottleneck in chromatography. Applications include sample preparation for dissolution testing, HPLC, UHPLC, UPLC® and liquid chromatography - mass spectrometry. It is currently available with 0.2µm or 0.45µm PTFE and PVDF philic Millex Samplicity filters. The Samplicity® filtration system includes a base, lid, vial tray, waste tray and tubing. ⚛ A High Performing UPLC System W aters’ Acquity UPLC® I-Class system is one of the highest performing UPLC systems, taking UltraPerformance LC® separations technolog y to the next level. The Acquity UPLC I-Class features the low system dispersion and carr yover. Low dispersion maximises peak c ­ apacity, thereby advancing chromatog raphic separations and optimising the p e r ­f o r m a n c e of any mass spectrometer. The I-Class s y stem e xcels when analysing a ny comple x , sample-limited compounds. These samples ca n represent complex separation challenges requiring an LC system that ca n ma x im ise the benef its of sub-2µ for faster throughput and optimised MS performance. Minimal system volume is a new key feature of the UPLC I-Class. Reduced system volume significantly decreases dispersion rates for reproducibly higher resolution and superior peak capacity, which extends the sensitivity of any mass spectrometer. Additionally, a low dispersion footprint allows users to reduce their separation cycle times without impact to the separation as the resolution is maintained even for ballistic gradients lasting less than one minute. It also features flexibility and precise sampling capabilities. Depending on their application needs, users can choose eit her t he highest precision and lowest dispersion fixed-loop sample manager or the world’s first low dispersion variable volume sa mple ma n a g er, w it h a f low-through needle design t h a t d e­l i v e r s h i gh-­p re c i sion injections, excellent sample recovery and low sample ca r r yover optimising the performance for even the most sensit ive mass detectors. ⚛ Microsep Contact: Louis van Huyssteen Tel: 011-553‑2300 Email: [email protected] Merck Millipore Field Marketing Manager: Adele Heath Tel: 011-372-5129 Email: [email protected] Cr(III) or Cr(VI)? T he determination of chromium in complex matrices is a notorious challenge, as interconversions between species may occur during sample preparation making quantif ication ver y difficult. In a recent study, Rahman et al performed speciated isotope dilution mass spectrometry (SIDMS), as described in EPA Method 6800 (update V), to determine chromium species in dietary supplements. EPA Method 6800 was implemented with a Metrohm ion chromatograph coupled to an Agilent mass spectrometer with inductively coupled plasma (IC-ICP-MS). Although Cr(III) and Cr(VI) are chemical forms of the same element, the effects of the two species on human health could not be more different. While Cr(III) is considered an essential trace metal found in many foods, Cr(VI) is a known carcinogenic with very strict limits applying to its presence in foods. The authors of the study point to the potential risk to consumers resulting from the fact that manufacturers of dietary supplements may not be aware of or even neglect the effects of possible interconversions of chromium species on the quality of the final products. The authors continue to present in detail the sample preparation/extraction methods required (EPA Method 3060A, EPA Method 3052) to make sure that subsequent determination of chromium species in solid samples is both accurate and reliable. The conclusion from the study is that ‘SIDMS [as per EPA Method 6800] facilitates simultaneous accounting of both Cr species concentrations and correction for transformations by enabling isotopic tagging for the oxidation of Cr(III) and the reduction of Cr(VI) during analysis in aqueous samples. The combined extraction/SIDMS procedure is capable of correcting for bidirectional species transformations that may occur during analyses of Cr(VI) in solid samples. ⚛