Chemistry Newsletter Fall 2017 | Page 11

ley Parr Robert as a ientist special who hrilling butions mistry... chemistry to Walter Kohn for his work on density func- tional theory and John Pople for his work on ab initio quantum chemistry. Catalyst–Oxide Assemblies An important element in synthetic organic chemistry has been the development and application of organic excited states in solution, either by sensitization or electron transfer catalysis. Exploitation of organic excited states has evolved from the bench scale to the photochemical reactor scale. Parr’s contributions to chemistry are characterized by his visionary approach and his foresight. In the speech at the American Chemical Society Southeast Regional Symposium in honor of Parr in 1998, Chemistry Nobel Prize winner John Pople summarized Parr’s contribu- tions: “I have followed Bob Parr’s footsteps through- out my career, starting from the field of semiempirical quantum chemistry to the latest effort in density func- tional theory.” In addition to his ground-breaking contributions to computational quantum theory, Parr was, of course, considered the father of conceptual DFT for chemistry, as clear- ly presented in the acclaimed Parr-Yang book, Density-Functional Theory of Atoms and Molecules, 1989. Robert Parr was a rare scientist and a special person who made thrilling contributions to chemistry while profoundly affecting the lives of the many young scientists whom he mentored and who have had contact with him and his work. In honor of Bob Parr’s scientific achievements and on the occa- sion of his 92nd birthday, an international conference “Frontiers of Theoretical Chemistry - the Parr Celebration,” was held in the Auditorium of French Family Science Center at Duke University, on Saturday, September 7, 2013. Over fifty participants, Parr’s scientific and international family and friends, gathered to pres- ent exciting new progress in the field Parr pioneered. There were over twenty presentations throughout the day. The meeting ended in the evening with a symposium dinner, where there were more speeches on reminiscences about Bob’s life and career. Obituary originally published in Angewandte Chemie, and is used by permission. In a parallel effort, with a different focus, advances have also been made in exploit- ing nanoparticle oxide surfaces for energy conversion applications based on chemi- cally bound molecular reactants, which has the advantage of maximization of the local microscopic surface volume for enhancing efficiencies. In a collaborative effort between the David Nicewicz and Thomas Meyer groups, pub- lished in PNAS, researchers describe the integration of the two areas with the goal of creating stable photochemical environ- ments that minimize reaction volumes in photooxidation reactions. The results pre- sented, provide a basis for extension to larger scales and to catalyst–oxide assem- blies with potential applications for larg- er-scale organic reactions.